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Water-Soluble Pentagonal-Prismatic Titanium-Oxo Clusters

Release time:2019-06-12 Hits:
Abstract:
By using solubility control to crystallize the prenucleation clusters of hydrosol, a family of titanium-oxo clusters possessing the {Ti18O27} core in which the 18 Ti(IV)-ions are uniquely connected with μ-oxo ligands into a triple-decked pentagonal prism was obtained. The cluster cores are wrapped by external sulfate and aqua ligands, showing good solubilities and stabilities in a variety of solvents including acetonitrile and water and allowing their solution chemistry being studied by means of electrospray ionization mass spectroscopy, 17O NMR, and vibrational spectroscopy. Furthermore, this
Correspondence Author:
Guanyun Zhang, Caiyun Liu, De-Liang Long, Leroy Cronin, Chen-Ho Tung, and Yifeng Wang*
Volume:
138
Issue:
35
Page Number:
11097–11100
Translation or Not:
no
Date of Publication:
2016-08-01