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何作利

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教授 博士生导师 硕士生导师

主要任职:无

其他任职:无

性别:男

毕业院校:西安交通大学&美国犹他大学联合培养

学历:博士研究生毕业

学位:工学博士学位

在职信息:在职

所在单位:环境科学与工程学院

入职时间:2019-06-14

学科:环境科学与工程
环境工程

办公地点:山东大学(青岛校区)会文南楼A座

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Multi-Walled Carbon Nanotubes Modified NiCo2S4 for the Efficient Photocatalytic Reduction of Hexavalent Chromium

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论文名称:Multi-Walled Carbon Nanotubes Modified NiCo2S4 for the Efficient Photocatalytic Reduction of Hexavalent Chromium

发表刊物:C-Journal of Carbon Research

刊物所在地:MDPI

关键字:photocatalysis; hexavalent chromium; NiCo2S4; CNT; reduction

摘要:Hexavalent chromium (Cr(VI)) compounds are considered to be occupational carcinogens, which can be transferred from the environment to the human body and pose a significant threat to human health. It is particularly urgent to explore a more efficient catalyst for removing Cr(VI) to comply with discharge standards. The addition of CNTs enables the separation and transfer of photogenerated charges. Thus, we synthesized a range of NiCo2S4 hybrid materials with different multi-walled carbon nanotube (MWCNTs) contents using a two-step hydrothermal method. The composites had significant advantages compared to pure NiCo2S4, such as an enhanced visible light absorption, increased specific surface area, high electron–hole pair separation, and fast electron transport. Thus, MWCNT addition enabled efficient photocatalytic performances in terms of reducing hexavalent chromium (Cr(VI)). Among all the composite samples, the MWCNT/NiCo2S4 with 0.050 g of MWCNTs achieved the highest efficiency in reducing Cr(VI) under light irradiation, which showed a removal rate close to 100% within 40 min. Such CNT-based composite photocatalysts could be used to reduce the highly toxic Cr(VI) in environmental applications.

第一作者:Qiu Jin

通讯作者:Zuoli He

全部作者:Ziye Zheng,Yuxiao Feng,Shuang Tian

论文类型:期刊论文

卷号:9

期号:4

页面范围:99

DOI码:10.3390/c9040099

字数:4000

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发表时间:2023-10

收录刊物:SCI

发布时间:2023-10-31