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发表刊物：J. Am. Chem. Soc.

摘要：Thecombinationof solutionself-assembly,whichenablesprimarymorphologicalcontrol,andsolidself-assembly,whichenablesthecreationof novelproperties,canleadto theformationof newfunctionalmaterialsthatcannotbe obtainedusingeithertechniquealone.Herein,we reporta cooperativesolution/solidself-assemblystrategyto  fabricatenoveltwo-dimensional(2D)platelets.Precursor2Dplateletswithpreor-ganizedpackingstructure,shape,andsizeare formedvia the livingself-assemblyof  a  donor−acceptorfluorophoreandvolatilecoformer(i.e.,propanol)in solutionphase.Afterhigh-temperatureannealing,propanolis releasedfromtheprecursorplatelets,andnewcontinuousintermolecularhydrogenbondsare formed.Thenew2Dplateletsformedretainthecontrollablemorphologiesoriginallydefinedby the solutionphaselivingself-assemblybut exhibitremarkableheat-resistantluminescenceup to 200°C  andhightwo-photonabsorptioncrosssections(i.e.,>19,000GMat 760nm laserexcitation).

第一作者：巩彦君

论文类型：文章

卷号：145

页面范围：9771

是否译文：否

发表时间：2023-04-01

收录刊物：SCI